Home / Articles / Optical properties of YSAG : Yb : Er ceramics with Sc3+ cations in the dodecahedral and octahedral positions of the garnet crystal lattice

Optical properties of YSAG : Yb : Er ceramics with Sc3+ cations in the dodecahedral and octahedral positions of the garnet crystal lattice

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1 North Caucasian Federal University, 1 Pushkin Str., Stavropol 355017, Russian Federation
2 Prokhorov General Physics Institute of the Russian Academy of Sciences, 38 Vavilov Str., Moscow 119991, Russian Federation
3 National University of Science and Technology “MISIS”, 4-1 Leninsky Ave., Moscow 119049, Russian Federation
10.3897/j.moem.9.3.115403
Published 12 October 2023
Communication , Volume 9, Issue 3, 133-144
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Tarala V. A. et al. Optical properties of YSAG : Yb : Er ceramics with Sc3+ cations in the dodecahedral and octahedral positions of the garnet crystal lattice // Modern Electronic Materials. 2023. Vol. 9. No. 3. pp. 133-144.
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Tarala V. A., Kravtsov A. A., Kuznetsov S. V., Malyavin F. F., Chapura O. M., Brazhko E. A., Kozhitov L. V. Optical properties of YSAG : Yb : Er ceramics with Sc3+ cations in the dodecahedral and octahedral positions of the garnet crystal lattice // Modern Electronic Materials. 2023. Vol. 9. No. 3. pp. 133-144.
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TY - JOUR
DO - 10.3897/j.moem.9.3.115403
UR - https://moem.colab.ws/publications/10.3897/j.moem.9.3.115403
TI - Optical properties of YSAG : Yb : Er ceramics with Sc3+ cations in the dodecahedral and octahedral positions of the garnet crystal lattice
T2 - Modern Electronic Materials
AU - Tarala, Vitaly A.
AU - Kravtsov, Alexander A.
AU - Kuznetsov, Sergey V.
AU - Malyavin, Fedor F.
AU - Chapura, Oleg M.
AU - Brazhko, Ekaterina A.
AU - Kozhitov, Lev V.
PY - 2023
DA - 2023/10/12
PB - НИТУ МИСИС
SP - 133-144
IS - 3
VL - 9
ER -
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@article{2023_Tarala,
author = {Vitaly A. Tarala and Alexander A. Kravtsov and Sergey V. Kuznetsov and Fedor F. Malyavin and Oleg M. Chapura and Ekaterina A. Brazhko and Lev V. Kozhitov},
title = {Optical properties of YSAG : Yb : Er ceramics with Sc3+ cations in the dodecahedral and octahedral positions of the garnet crystal lattice},
journal = {Modern Electronic Materials},
year = {2023},
volume = {9},
publisher = {НИТУ МИСИС},
month = {Oct},
url = {https://moem.colab.ws/publications/10.3897/j.moem.9.3.115403},
number = {3},
pages = {133--144},
doi = {10.3897/j.moem.9.3.115403}
}
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Tarala, Vitaly A., et al. “Optical properties of YSAG : Yb : Er ceramics with Sc3+ cations in the dodecahedral and octahedral positions of the garnet crystal lattice.” Modern Electronic Materials, vol. 9, no. 3, Oct. 2023, pp. 133-144. https://moem.colab.ws/publications/10.3897/j.moem.9.3.115403.
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Keywords

ceramics
luminescence
Optical properties
solid solution
yttrium scandium aluminum garnet

Abstract

Optical ceramics based on YSAG : Yb : Er with the compositions {Y1.86Yb0.45Er0.09Sc0.6}[Al1.6Sc0.4]Al3O12 and {Y2.26Yb0.45Er0.09Sc0.2}[Al1.0Sc1.0]Al3O12 were fabricated by vacuum sintering from pre-synthesized nanocrystalline powders. A comparative analysis of these samples with optical ceramics of the compositions {Y2.34Yb0.45Er0.09Sc0.12}[Al1.92Sc0.08]Al3O12 and {Y0.96Yb0.45Er0.09Sc1.50}[Al1.8Sc0.2]Al3O12 was carried out. The influence of scandium cations in the dodecahedral and octahedral positions of the garnet crystal lattice on the refractive index of YSAG : Yb : Er, as well as the values of absorption coefficients, integral luminescent intensities, and lifetimes of excited states of Yb3+ (2F7/2 and 2F5/2) and Er3+ (4I15/2, 4I13/2, 4F9/2, and 4S3/2) cations was revealed in the wavelength ranges 520–700 nm and 890–1690 nm. It has been shown that by changing the concentrations of scandium cations in the dodecahedral and octahedral positions of the crystal lattice of YSAG : Yb : Er solid solutions, it is possible to purposefully change the efficiency of energy transfer from ytterbium cations to erbium cations.

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